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We theoretically and computationally study the generation of high-order harmonics in the water window from a semi-infinite gas cell where a few-cycle, carrier-envelope-phase-controlled 1.7-µm driving laser pulse undergoes nonlinear propagation via optical Kerr effect (self-focusing) and plasma defocusing. Our calculation shows that high harmonic signals are enhanced for extended propagation distances and furthermore, isolated attosecond pulses in the water window can be generated from the semi-infinite gas cell. This enhancement is attributed mainly to better phase matching for extended propagation distances achieved via nonlinear propagation and resulting intensity stabilization.more » « less
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Dempsey, Dennis; Nagar, Garima_C; Renskers, Christopher_K; Grynko, Rostislav_I; Sutherland, James_S; Shim, Bonggu (, Optics Letters)We perform single-shot frequency domain holography to measure the ultrafast spatio-temporal phase change induced by the optical Kerr effect and plasma in flexible Corning Willow Glass during femtosecond laser–matter interactions. We measure the nonlinear index of refraction ( ) to be and visualize the plasma formation and recombination on femtosecond time scales in a single shot. To compare with the experiment, we carry out numerical simulations by solving the nonlinear envelope equation.more » « less
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